Abstract
Exploiting the polarization properties of coherent Raman scattering in liquids, new techniques of polarization-controlled 3-colour CARS are described. It is shown that the nonresonant, resonant-isotropic and resonant-anisotropic scattering components can be alternatively eliminated for special geometries with magic angles of the polarization of the detected anti-Stokes signal. Perturbations via the optical Kerr effect are discussed. The potential to study the molecular reorientational motion and isolated dephasing channels is demonstrated.
| Original language | English |
|---|---|
| Pages (from-to) | 979-988 |
| Number of pages | 10 |
| Journal | Il Nuovo Cimento D |
| Volume | 14 |
| Issue number | 10 |
| DOIs | |
| State | Published - Oct 1992 |
| Externally published | Yes |
Keywords
- CARS
- Stimulated Raman scattering and spectra
- Time-resolved optical spectroscopies and other ultrafast optical measurements in condensed matter
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