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Time domain coherent Raman techniques

  • Universität Bayreuth

Research output: Contribution to journalArticlepeer-review

7 Scopus citations

Abstract

Exploiting the polarization properties of coherent Raman scattering in liquids, new techniques of polarization-controlled 3-colour CARS are described. It is shown that the nonresonant, resonant-isotropic and resonant-anisotropic scattering components can be alternatively eliminated for special geometries with magic angles of the polarization of the detected anti-Stokes signal. Perturbations via the optical Kerr effect are discussed. The potential to study the molecular reorientational motion and isolated dephasing channels is demonstrated.

Original languageEnglish
Pages (from-to)979-988
Number of pages10
JournalIl Nuovo Cimento D
Volume14
Issue number10
DOIs
StatePublished - Oct 1992
Externally publishedYes

Keywords

  • CARS
  • Stimulated Raman scattering and spectra
  • Time-resolved optical spectroscopies and other ultrafast optical measurements in condensed matter

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