Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

M. F. Gelin; A. V. Pisliakov; W. Domcke

doi:10.1103/PhysRevA.65.062507

Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

M. F. Gelin, A. V. Pisliakov, W. Domcke

Chair of Theoretical Chemistry

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36 Scopus citations

Abstract

Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

Original language	English
Article number	062507
Pages (from-to)	625071-6250714
Number of pages	5625644
Journal	Physical Review A
Volume	65
Issue number	6
DOIs	https://doi.org/10.1103/PhysRevA.65.062507
State	Published - Jun 2002

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10.1103/PhysRevA.65.062507

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title = "Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state",

abstract = "Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.",

author = "Gelin, {M. F.} and Pisliakov, {A. V.} and W. Domcke",

year = "2002",

month = jun,

doi = "10.1103/PhysRevA.65.062507",

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journal = "Physical Review A",

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AU - Pisliakov, A. V.

AU - Domcke, W.

PY - 2002/6

Y1 - 2002/6

N2 - Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

AB - Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

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U2 - 10.1103/PhysRevA.65.062507

DO - 10.1103/PhysRevA.65.062507

M3 - Article

AN - SCOPUS:0036599742

SN - 1050-2947

VL - 65

SP - 625071

EP - 6250714

JO - Physical Review A

JF - Physical Review A

IS - 6

M1 - 062507

ER -

Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

Abstract

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