The capacity of the Hg/HClO4 • 5.5H2O interface in the liquid-liquid, solid-liquid and solid-solid state temperature and potential dependence

Marcella Cappadonia, H. Thomas Von Der Heyden, Ulrich Stimming

Research output: Contribution to journalArticlepeer-review

2 Scopus citations

Abstract

The interface Hg/HClO4 • 5.5H2O was investigated by cyclic voltammetry and electrochemical impedance spectroscopy between 170 and 300 K. In this temperature range, phase transitions occur for electrode and electrolyte, such that within 6 K the electrode-electrolyte interface changes from solid-solid over solid-liquid to liquid-liquid or vice versa. The double layer capacity was investigated as a function of potential for different temperatures and states of aggregation of the respective phases.

Original languageEnglish
Pages (from-to)9-16
Number of pages8
JournalSolid State Ionics
Volume94
Issue number1-4
DOIs
StatePublished - 1 Feb 1997
Externally publishedYes

Keywords

  • Double layer capacity
  • Electrode-electrolyte interface

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