TY - JOUR
T1 - Quantitative comparability of heavy ion and in-pile irradiations on UMo fuel systems
AU - Breitkreutz, Harald
AU - Heldmann, Alexander
AU - Hingerl, Jürgen
AU - Jungwirth, Rainer
AU - Shi, Jingyi
AU - Petry, Winfried
N1 - Publisher Copyright:
© 2018 Elsevier B.V.
PY - 2018/8/15
Y1 - 2018/8/15
N2 - Irradiation with heavy ions is an increasingly often used tool to quickly reproduce and simulate certain effects of irradiation tests in nuclear reactors (in-pile irradiations). Using SRIM/TRIM, a dataset for the deposition of energy and the creation of vacancies in UMo/Al fuels by in-pile fission products as well as out-of-pile Iodine-127 ions (80 Mev) has been created, that allows for a proportional conversion of ion flux and fluency in the corresponding fission rate and burn-up equivalents. The conversion factor depends on the irradiated geometry, i. e. order of the layers and thickness of the top layer, as well as on the point of interest in the sample. To verify the calculations, a comparison of thicknesses and growth dynamics of out-of-pile produced interdiffusion layers (IDL) with predictions based on in-pile data has been made. The IDL is mainly composed of UAlx and forms during irradiation at the UMo-Al-interface. The observed thicknesses match within 10%, which is well inside the uncertainties of both methods. This demonstrates the applicability of the presented conversion approach as well as the reliability of heavy ion irradiations. The data from two I-127 irradiation experiments furthermore support the current understanding of the Arrhenius-like in-pile IDL growth, i. e. its forth-root dependency on fission rate (or ion flux), the square-root dependency on the irradiation time and the exponential temperature dependency.
AB - Irradiation with heavy ions is an increasingly often used tool to quickly reproduce and simulate certain effects of irradiation tests in nuclear reactors (in-pile irradiations). Using SRIM/TRIM, a dataset for the deposition of energy and the creation of vacancies in UMo/Al fuels by in-pile fission products as well as out-of-pile Iodine-127 ions (80 Mev) has been created, that allows for a proportional conversion of ion flux and fluency in the corresponding fission rate and burn-up equivalents. The conversion factor depends on the irradiated geometry, i. e. order of the layers and thickness of the top layer, as well as on the point of interest in the sample. To verify the calculations, a comparison of thicknesses and growth dynamics of out-of-pile produced interdiffusion layers (IDL) with predictions based on in-pile data has been made. The IDL is mainly composed of UAlx and forms during irradiation at the UMo-Al-interface. The observed thicknesses match within 10%, which is well inside the uncertainties of both methods. This demonstrates the applicability of the presented conversion approach as well as the reliability of heavy ion irradiations. The data from two I-127 irradiation experiments furthermore support the current understanding of the Arrhenius-like in-pile IDL growth, i. e. its forth-root dependency on fission rate (or ion flux), the square-root dependency on the irradiation time and the exponential temperature dependency.
KW - Burn-up
KW - Heavy ion irradiation
KW - Interdiffusion layer
KW - SRIM
KW - UMo
UR - http://www.scopus.com/inward/record.url?scp=85046999145&partnerID=8YFLogxK
U2 - 10.1016/j.jnucmat.2018.04.007
DO - 10.1016/j.jnucmat.2018.04.007
M3 - Article
AN - SCOPUS:85046999145
SN - 0022-3115
VL - 507
SP - 276
EP - 287
JO - Journal of Nuclear Materials
JF - Journal of Nuclear Materials
ER -