New results on vibrational population decay in simple liquids

H. Graener; A. Laubereau

doi:10.1007/BF00688670

New results on vibrational population decay in simple liquids

H. Graener, A. Laubereau

Universität Bayreuth

Research output: Contribution to journal › Article › peer-review

52 Scopus citations

Abstract

The population lifetimes of the symmetric CH₂-stretching mode of several methylene halides were measured after infrared excitation by spontaneous anti-Stokes Raman scattering of delayed picosecond probe pulses. Data ranging from 6.5 to 45 ps are reported. The results give evidence for vibrational energy transfer via anharmonic coupling to neighbouring vibrational combination bands and overtones.

Original language	English
Pages (from-to)	213-218
Number of pages	6
Journal	Applied Physics B Photophysics and Laser Chemistry
Volume	29
Issue number	3
DOIs	https://doi.org/10.1007/BF00688670
State	Published - Nov 1982
Externally published	Yes

Keywords

07.65
34
35

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10.1007/BF00688670

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title = "New results on vibrational population decay in simple liquids",

abstract = "The population lifetimes of the symmetric CH2-stretching mode of several methylene halides were measured after infrared excitation by spontaneous anti-Stokes Raman scattering of delayed picosecond probe pulses. Data ranging from 6.5 to 45 ps are reported. The results give evidence for vibrational energy transfer via anharmonic coupling to neighbouring vibrational combination bands and overtones.",

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author = "H. Graener and A. Laubereau",

year = "1982",

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language = "English",

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AU - Graener, H.

AU - Laubereau, A.

PY - 1982/11

Y1 - 1982/11

N2 - The population lifetimes of the symmetric CH2-stretching mode of several methylene halides were measured after infrared excitation by spontaneous anti-Stokes Raman scattering of delayed picosecond probe pulses. Data ranging from 6.5 to 45 ps are reported. The results give evidence for vibrational energy transfer via anharmonic coupling to neighbouring vibrational combination bands and overtones.

AB - The population lifetimes of the symmetric CH2-stretching mode of several methylene halides were measured after infrared excitation by spontaneous anti-Stokes Raman scattering of delayed picosecond probe pulses. Data ranging from 6.5 to 45 ps are reported. The results give evidence for vibrational energy transfer via anharmonic coupling to neighbouring vibrational combination bands and overtones.

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DO - 10.1007/BF00688670

M3 - Article

AN - SCOPUS:0020205721

SN - 0721-7269

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EP - 218

JO - Applied Physics B Photophysics and Laser Chemistry

JF - Applied Physics B Photophysics and Laser Chemistry

IS - 3

ER -

New results on vibrational population decay in simple liquids

Abstract

Keywords

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