TY - JOUR
T1 - Multistate Nonvolatile Metamirrors with Tunable Optical Chirality
AU - Huang, Yijia
AU - Xiao, Tianxiao
AU - Xie, Zhengwei
AU - Zheng, Jie
AU - Su, Yarong
AU - Chen, Weidong
AU - Liu, Ke
AU - Tang, Mingjun
AU - Zhu, Jianqi
AU - Müller-Buschbaum, Peter
AU - Li, Ling
N1 - Publisher Copyright:
© 2021 American Chemical Society
PY - 2021/9/29
Y1 - 2021/9/29
N2 - Compared with conventional mirrors that behave as isotropic electromagnetic (EM) reflectors, metamirrors composed of periodically aligned artificial meta-atoms exhibit increased degrees of freedom for EM manipulations. However, the functionality of most metamirrors is fixed by design, and how to achieve active EM control is still elusive. Here, we propose a multistate metamirror based on the nonvolatile phase change material Ge2Sb2Te5(GST) with four distinct functionalities that can be realized in the infrared region by exploiting the temperature-activated phase transition. When varying the crystallinity of GST, the metamirror has the capability to perform as a right-handed circular polarization chiral mirror, a narrowband achiral mirror, a left-handed circular polarization chiral mirror, or a broadband achiral mirror, respectively. The inner physics is further explained by the construction or cancellation of extrinsic two-dimensional chirality. As a proof of concept, experimental verification is carried out and the measured results agree well with their simulated counterparts. Such a multifunctional tunable metamirror could address a wide range of applications from sensing and spectroscopy to analytical chemistry and imaging.
AB - Compared with conventional mirrors that behave as isotropic electromagnetic (EM) reflectors, metamirrors composed of periodically aligned artificial meta-atoms exhibit increased degrees of freedom for EM manipulations. However, the functionality of most metamirrors is fixed by design, and how to achieve active EM control is still elusive. Here, we propose a multistate metamirror based on the nonvolatile phase change material Ge2Sb2Te5(GST) with four distinct functionalities that can be realized in the infrared region by exploiting the temperature-activated phase transition. When varying the crystallinity of GST, the metamirror has the capability to perform as a right-handed circular polarization chiral mirror, a narrowband achiral mirror, a left-handed circular polarization chiral mirror, or a broadband achiral mirror, respectively. The inner physics is further explained by the construction or cancellation of extrinsic two-dimensional chirality. As a proof of concept, experimental verification is carried out and the measured results agree well with their simulated counterparts. Such a multifunctional tunable metamirror could address a wide range of applications from sensing and spectroscopy to analytical chemistry and imaging.
KW - chirality
KW - circular dichroism
KW - metamirror
KW - multifunctional
KW - phase change material
UR - http://www.scopus.com/inward/record.url?scp=85116063076&partnerID=8YFLogxK
U2 - 10.1021/acsami.1c14204
DO - 10.1021/acsami.1c14204
M3 - Article
C2 - 34520183
AN - SCOPUS:85116063076
SN - 1944-8244
VL - 13
SP - 45890
EP - 45897
JO - ACS Applied Materials and Interfaces
JF - ACS Applied Materials and Interfaces
IS - 38
ER -