Longitudinal Neutron Resonance Spin Echo Spectroscopy under Large Energy Transfers

Longitudinal neutron resonance spin echo (LNRSE) spectroscopy offers very high energy resolution due to the self correction of the resonant spin flippers, and a wide dynamical range nominally exceeding six orders of magnitude in resolution down to sub-ps range. In this paper, the technical realisation how to achieve such low Fourier times at the spectrometer RESEDA at the MLZ Garching is described. The requirements of data collection and data analysis in the limit of very low Fourier times, notably those related to the breakdown of the spin echo approximation, are discussed. A method to infer the scattering function from the experimental data under large energy tansfers beyond the spin echo approximation is presented.