Infrared identification of the FCS radical in an argon matrix

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Abstract

The FCS radical has been produced using a pulsed-jet DC discharge technique with several precursor molecules and characterized by IR absorption spectroscopy in an argon matrix. The spectra were analyzed and the following vibrational assignments, confirmed by isotopic studies, and by normal coordinate analysis were determined: ν1 = 1297.9 cm-1, 2ν2 = 910.3 cm-1 in Fermi resonance with ν3 = 917.9 cm-1, and ν1 + ν3 = 2202.6 cm-1 in Fermi resonance with 2ν2 + ν3 = 2195.7 cm-1.

Original languageEnglish
Pages (from-to)329-339
Number of pages11
JournalChemical Physics Letters
Volume212
Issue number3-4
DOIs
StatePublished - 10 Sep 1993

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