Crystal growth and thermodynamic properties of (Ca, La) 14Cu24O41

U. Ammerahl, C. Kerpen, B. Büchner, R. Gross, H. Micklitz, A. Revcolevschi

Research output: Contribution to journalArticlepeer-review

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Abstract

High quality, centimeter size single crystals of Ca14-xLaxCu24O41 have been successfully grown using the travelling solvent floating zone (TSFZ) method in association with an image furnace. Crystals grown under oxygen pressures up to 13 bar are single phase for 2 ≤ x ≤ 5. Growth initiated on a single crystalline seed, in combination with an appropriate solvent disk, yields a single domain almost directly from the beginning of the growth. Crystals were characterized by EDX, TGA and X-ray powder diffraction. In addition magnetic susceptibility and specific heat measurements were performed. Long range antiferromagnetic order occurs at TN=9.7 K for xLa = 5, whereas for lower La concentrations TN is considerably suppressed.

Original languageEnglish
Pages (from-to)723-727
Number of pages5
JournalJournal of Low Temperature Physics
Volume117
Issue number3-4
DOIs
StatePublished - 1999
Externally publishedYes

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