Compact phase-stable design for single- And double-quantum two-dimensional electronic spectroscopy

Alexandra Nemeth; Jaroslaw Sperling; Jürgen Hauer; Harald F. Kauffmann; Franz Milota

doi:10.1364/OL.34.003301

Compact phase-stable design for single- And double-quantum two-dimensional electronic spectroscopy

Alexandra Nemeth, Jaroslaw Sperling, Jürgen Hauer, Harald F. Kauffmann, Franz Milota

Research output: Contribution to journal › Article › peer-review

41 Scopus citations

Abstract

We report a compact, easy to align, and passively phase-stabilized setup for recording two-dimensional (2D) electronic spectra in three different phase-matching directions in the boxcar geometry. Passive phase stabilization is achieved by a diffractive optical element, the use of refractive optics for introducing pulse delays, and the use of common optics for all pulses. Representative 2D spectra correlating single- and doublequantum coherences in a molecular aggregate are presented.

Original language	English
Pages (from-to)	3301-3303
Number of pages	3
Journal	Optics Letters
Volume	34
Issue number	21
DOIs	https://doi.org/10.1364/OL.34.003301
State	Published - 1 Nov 2009
Externally published	Yes

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abstract = "We report a compact, easy to align, and passively phase-stabilized setup for recording two-dimensional (2D) electronic spectra in three different phase-matching directions in the boxcar geometry. Passive phase stabilization is achieved by a diffractive optical element, the use of refractive optics for introducing pulse delays, and the use of common optics for all pulses. Representative 2D spectra correlating single- and doublequantum coherences in a molecular aggregate are presented.",

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AU - Kauffmann, Harald F.

AU - Milota, Franz

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AB - We report a compact, easy to align, and passively phase-stabilized setup for recording two-dimensional (2D) electronic spectra in three different phase-matching directions in the boxcar geometry. Passive phase stabilization is achieved by a diffractive optical element, the use of refractive optics for introducing pulse delays, and the use of common optics for all pulses. Representative 2D spectra correlating single- and doublequantum coherences in a molecular aggregate are presented.

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Compact phase-stable design for single- And double-quantum two-dimensional electronic spectroscopy

Abstract

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