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Coherent pulse propagation in the infrared on the picosecond time scale

  • Universität Bayreuth

Research output: Contribution to journalArticlepeer-review

37 Scopus citations

Abstract

Coherent propagation of resonant ultrashort pulses in gases is investigated theoretically and experimentally at medium pressure values. Drastic changes of the pulse wings extending over several ten picoseconds are predicted and experimentally observed using tunable pulses of 4 ps produced by a parametric generator device and picosecond IR light gates. The dephasing time T2 of the R(3) vibration-rotation transition of HCl is measured to be T2 × p = 21.5 ps × bar in the pressure range p = 1 to 3 bar. Quantitative agreement between theory and experiment demonstrates that a novel transient spectroscopy in the infrared can be accomplished by coherent pulse reshaping.

Original languageEnglish
Pages (from-to)117-122
Number of pages6
JournalOptics Communications
Volume47
Issue number2
DOIs
StatePublished - 15 Aug 1983
Externally publishedYes

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