A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces

E. Magerl; S. Neppl; A. L. Cavalieri; E. M. Bothschafter; M. Stanislawski; Th Uphues; M. Hofstetter; U. Kleineberg; J. V. Barth; D. Menzel; F. Krausz; R. Ernstorfer; R. Kienberger; P. Feulner

doi:10.1063/1.3596564

A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces

E. Magerl, S. Neppl, A. L. Cavalieri, E. M. Bothschafter, M. Stanislawski, Th Uphues, M. Hofstetter, U. Kleineberg, J. V. Barth, D. Menzel, F. Krausz, R. Ernstorfer, R. Kienberger, P. Feulner

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Abstract

We describe an apparatus for attosecond photoelectron spectroscopy of solids and surfaces, which combines the generation of isolated attosecond extreme-ultraviolet (XUV) laser pulses by high harmonic generation in gases with time-resolved photoelectron detection and surface science techniques in an ultrahigh vacuum environment. This versatile setup provides isolated attosecond pulses with photon energies of up to 140 eV and few-cycle near infrared pulses for studying ultrafast electron dynamics in a large variety of surfaces and interfaces. The samples can be prepared and characterized on an atomic scale in a dedicated flexible surface science end station. The extensive possibilities offered by this apparatus are demonstrated by applying attosecond XUV pulses with a central photon energy of ∼125 eV in an attosecond streaking experiment of a xenon multilayer grown on a Re(0001) substrate.

Original language	English
Article number	063104
Journal	Review of Scientific Instruments
Volume	82
Issue number	6
DOIs	https://doi.org/10.1063/1.3596564
State	Published - Jun 2011

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Magerl, E., Neppl, S., Cavalieri, A. L., Bothschafter, E. M., Stanislawski, M., Uphues, T., Hofstetter, M., Kleineberg, U., Barth, J. V., Menzel, D., Krausz, F., Ernstorfer, R., Kienberger, R., & Feulner, P. (2011). A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces. Review of Scientific Instruments, 82(6), Article 063104. https://doi.org/10.1063/1.3596564

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title = "A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces",

abstract = "We describe an apparatus for attosecond photoelectron spectroscopy of solids and surfaces, which combines the generation of isolated attosecond extreme-ultraviolet (XUV) laser pulses by high harmonic generation in gases with time-resolved photoelectron detection and surface science techniques in an ultrahigh vacuum environment. This versatile setup provides isolated attosecond pulses with photon energies of up to 140 eV and few-cycle near infrared pulses for studying ultrafast electron dynamics in a large variety of surfaces and interfaces. The samples can be prepared and characterized on an atomic scale in a dedicated flexible surface science end station. The extensive possibilities offered by this apparatus are demonstrated by applying attosecond XUV pulses with a central photon energy of ∼125 eV in an attosecond streaking experiment of a xenon multilayer grown on a Re(0001) substrate.",

author = "E. Magerl and S. Neppl and Cavalieri, {A. L.} and Bothschafter, {E. M.} and M. Stanislawski and Th Uphues and M. Hofstetter and U. Kleineberg and Barth, {J. V.} and D. Menzel and F. Krausz and R. Ernstorfer and R. Kienberger and P. Feulner",

note = "Funding Information: The authors thank K. K{\"o}lbl, K. Eberle, and H. P. Sch{\"o}nauer for their valuable contributions to this work. Supported by the DFG Cluster of Excellence: Munich Centre for Advanced Photonics ( www.munich-photonics.de ). R.K. acknowledges funding from the Sofja Kovalevskaja Award of the Alexander von Humboldt Foundation and an ERC Starting Grant.",

year = "2011",

month = jun,

doi = "10.1063/1.3596564",

language = "English",

volume = "82",

journal = "Review of Scientific Instruments",

issn = "0034-6748",

publisher = "American Institute of Physics",

number = "6",

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Magerl, E, Neppl, S, Cavalieri, AL, Bothschafter, EM, Stanislawski, M, Uphues, T, Hofstetter, M, Kleineberg, U, Barth, JV, Menzel, D, Krausz, F, Ernstorfer, R, Kienberger, R & Feulner, P 2011, 'A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces', Review of Scientific Instruments, vol. 82, no. 6, 063104. https://doi.org/10.1063/1.3596564

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AU - Magerl, E.

AU - Neppl, S.

AU - Cavalieri, A. L.

AU - Bothschafter, E. M.

AU - Stanislawski, M.

AU - Uphues, Th

AU - Hofstetter, M.

AU - Kleineberg, U.

AU - Barth, J. V.

AU - Menzel, D.

AU - Krausz, F.

AU - Ernstorfer, R.

AU - Kienberger, R.

AU - Feulner, P.

N1 - Funding Information: The authors thank K. Kölbl, K. Eberle, and H. P. Schönauer for their valuable contributions to this work. Supported by the DFG Cluster of Excellence: Munich Centre for Advanced Photonics ( www.munich-photonics.de ). R.K. acknowledges funding from the Sofja Kovalevskaja Award of the Alexander von Humboldt Foundation and an ERC Starting Grant.

PY - 2011/6

Y1 - 2011/6

N2 - We describe an apparatus for attosecond photoelectron spectroscopy of solids and surfaces, which combines the generation of isolated attosecond extreme-ultraviolet (XUV) laser pulses by high harmonic generation in gases with time-resolved photoelectron detection and surface science techniques in an ultrahigh vacuum environment. This versatile setup provides isolated attosecond pulses with photon energies of up to 140 eV and few-cycle near infrared pulses for studying ultrafast electron dynamics in a large variety of surfaces and interfaces. The samples can be prepared and characterized on an atomic scale in a dedicated flexible surface science end station. The extensive possibilities offered by this apparatus are demonstrated by applying attosecond XUV pulses with a central photon energy of ∼125 eV in an attosecond streaking experiment of a xenon multilayer grown on a Re(0001) substrate.

AB - We describe an apparatus for attosecond photoelectron spectroscopy of solids and surfaces, which combines the generation of isolated attosecond extreme-ultraviolet (XUV) laser pulses by high harmonic generation in gases with time-resolved photoelectron detection and surface science techniques in an ultrahigh vacuum environment. This versatile setup provides isolated attosecond pulses with photon energies of up to 140 eV and few-cycle near infrared pulses for studying ultrafast electron dynamics in a large variety of surfaces and interfaces. The samples can be prepared and characterized on an atomic scale in a dedicated flexible surface science end station. The extensive possibilities offered by this apparatus are demonstrated by applying attosecond XUV pulses with a central photon energy of ∼125 eV in an attosecond streaking experiment of a xenon multilayer grown on a Re(0001) substrate.

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A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces

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