TY - JOUR
T1 - Universal and nonuniversal features of glassy relaxation in propylene carbonate
AU - Götze, W.
AU - Voigtmann, Th
PY - 2000
Y1 - 2000
N2 - It is demonstrated that the susceptibility spectra of supercooled propylene carbonate as measured by depolarized-light scattering, dielectric-loss, and incoherent quasielastic neutron-scattering spectroscopy within the GHz window are simultaneously described by the solutions of a two-component schematic model of the mode-coupling theory (MCT) for the evolution of glassy dynamics. It is shown that the universal [Formula Presented]-relaxation-scaling laws, dealing with the asymptotic behavior of the MCT solutions, describe the qualitative features of the calculated spectra. But the nonuniversal corrections to the scaling laws render it impossible to achieve a complete quantitative description using only the leading-order-asymptotic results.
AB - It is demonstrated that the susceptibility spectra of supercooled propylene carbonate as measured by depolarized-light scattering, dielectric-loss, and incoherent quasielastic neutron-scattering spectroscopy within the GHz window are simultaneously described by the solutions of a two-component schematic model of the mode-coupling theory (MCT) for the evolution of glassy dynamics. It is shown that the universal [Formula Presented]-relaxation-scaling laws, dealing with the asymptotic behavior of the MCT solutions, describe the qualitative features of the calculated spectra. But the nonuniversal corrections to the scaling laws render it impossible to achieve a complete quantitative description using only the leading-order-asymptotic results.
UR - http://www.scopus.com/inward/record.url?scp=0000820483&partnerID=8YFLogxK
U2 - 10.1103/PhysRevE.61.4133
DO - 10.1103/PhysRevE.61.4133
M3 - Article
AN - SCOPUS:0000820483
SN - 1063-651X
VL - 61
SP - 4133
EP - 4147
JO - Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
JF - Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
IS - 4
ER -