Ultrafast charge transfer visualized by two-dimensional electronic spectroscopy

O. Bixner, N. Christensson, J. Hauer, F. Milota, T. Mančal, V. Lukeš, H. F. Kauffmann

Publikation: Beitrag in Buch/Bericht/KonferenzbandKonferenzbeitragBegutachtung

Abstract

Two-dimensional electronic spectroscopy (2D-ES) is used to investigate ultrafast excited-state dynamics in a lutetium bisphthalocyanine dimer. Following optical excitation, a chain of electron and hole transfer steps gives rise to characteristic cross-peak dynamics in the electronic 2D spectra. The combination of density matrix propagation and quantum chemical calculations results in a molecular view of the charge transfer dynamics and highlights the role of the counter-ion in providing an energetic perturbation which promotes charge transfer across the complex.

OriginalspracheEnglisch
Titel18th International Conference on Ultrafast Phenomena, UP 2012
DOIs
PublikationsstatusVeröffentlicht - 2013
Extern publiziertJa
Veranstaltung18th International Conference on Ultrafast Phenomena, UP 2012 - Lausanne, Schweiz
Dauer: 8 Juli 201213 Juli 2012

Publikationsreihe

NameEPJ Web of Conferences
Band41
ISSN (Print)2101-6275
ISSN (elektronisch)2100-014X

Konferenz

Konferenz18th International Conference on Ultrafast Phenomena, UP 2012
Land/GebietSchweiz
OrtLausanne
Zeitraum8/07/1213/07/12

Fingerprint

Untersuchen Sie die Forschungsthemen von „Ultrafast charge transfer visualized by two-dimensional electronic spectroscopy“. Zusammen bilden sie einen einzigartigen Fingerprint.

Dieses zitieren