Time- and frequency-resolved fluorescence with a single TCSPC detector via a Fourier-transform approach

Antonio Perri, John H. Gaida, Andrea Farina, Fabrizio Preda, Daniele Viola, Matteo Ballottari, Jürgen Hauer, Sandro D.E. Silvestri, Cosimo D’Andrea, Giulio Cerullo, Dario Polli

Publikation: Beitrag in FachzeitschriftArtikelBegutachtung

22 Zitate (Scopus)

Abstract

We introduce a broadband single-pixel spectro-temporal fluorescence detector, combining time-correlated single photon counting (TCSPC) with Fourier transform (FT) spectroscopy. A birefringent common-path interferometer (CPI) generates two time-delayed replicas of the sample’s fluorescence. Via FT of their interference signal at the detector, we obtain a two-dimensional map of the fluorescence as a function of detection wavelength and emission time, with high temporal and spectral resolution. Our instrument is remarkably simple, as it only requires the addition of a CPI to a standard single-pixel TCSPC system, and it shows a readily adjustable spectral resolution with inherently broad bandwidth coverage.

OriginalspracheEnglisch
Seiten (von - bis)2270-2279
Seitenumfang10
FachzeitschriftOptics Express
Jahrgang26
Ausgabenummer3
DOIs
PublikationsstatusVeröffentlicht - 5 Feb. 2018

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