Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

M. F. Gelin; A. V. Pisliakov; W. Domcke

doi:10.1103/PhysRevA.65.062507

Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

M. F. Gelin
, A. V. Pisliakov
, W. Domcke

Lehrstuhl für Theoretische Chemie

Natl. Academy of Sciences of Belarus
Technische Universität München

Publikation: Beitrag in Fachzeitschrift › Artikel › Begutachtung

42 Zitate (Scopus)

Abstract

Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

Originalsprache	Englisch
Aufsatznummer	062507
Seiten (von - bis)	625071-6250714
Seitenumfang	5625644
Fachzeitschrift	Physical Review A
Jahrgang	65
Ausgabenummer	6
DOIs	https://doi.org/10.1103/PhysRevA.65.062507
Publikationsstatus	Veröffentlicht - Juni 2002

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10.1103/PhysRevA.65.062507

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title = "Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state",

abstract = "Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.",

author = "Gelin, \{M. F.\} and Pisliakov, \{A. V.\} and W. Domcke",

year = "2002",

month = jun,

doi = "10.1103/PhysRevA.65.062507",

language = "English",

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journal = "Physical Review A",

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N2 - Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

AB - Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.

UR - https://www.scopus.com/pages/publications/0036599742

U2 - 10.1103/PhysRevA.65.062507

DO - 10.1103/PhysRevA.65.062507

M3 - Article

AN - SCOPUS:0036599742

SN - 1050-2947

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SP - 625071

EP - 6250714

JO - Physical Review A

JF - Physical Review A

IS - 6

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Time- and frequency-gated spontaneous emission as a tool for studying vibrational dynamics in the excited state

Abstract

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