Abstract
Time and frequency-gated (TFG) spontaneous emission (SE) was discussed as a tool for studying vibrational dynamics in the excited state. The doorway-window picture of temporally and spectrally resolved spectra was developed. It was found that the TFG SE spectrum carried information on the strength of the system-bath coupling and the relative magnitude of the bath correlation time.
| Originalsprache | Englisch |
|---|---|
| Aufsatznummer | 062507 |
| Seiten (von - bis) | 625071-6250714 |
| Seitenumfang | 5625644 |
| Fachzeitschrift | Physical Review A |
| Jahrgang | 65 |
| Ausgabenummer | 6 |
| DOIs | |
| Publikationsstatus | Veröffentlicht - Juni 2002 |