Perspectives of shaped pulses for EPR spectroscopy

Philipp E. Spindler; Philipp Schöps; Wolfgang Kallies; Steffen J. Glaser; Thomas F. Prisner

doi:10.1016/j.jmr.2017.02.023

Perspectives of shaped pulses for EPR spectroscopy

Philipp E. Spindler, Philipp Schöps, Wolfgang Kallies, Steffen J. Glaser, Thomas F. Prisner

Professur für Organische Chemie

Publikation: Beitrag in Fachzeitschrift › Artikel › Begutachtung

61 Zitate (Scopus)

Abstract

This article describes current uses of shaped pulses, generated by an arbitrary waveform generator, in the field of EPR spectroscopy. We show applications of sech/tanh and WURST pulses to dipolar spectroscopy, including new pulse schemes and procedures, and discuss the more general concept of optimum-control-based pulses for applications in EPR spectroscopy. The article also describes a procedure to correct for experimental imperfections, mostly introduced by the microwave resonator, and discusses further potential applications and limitations of such pulses.

Originalsprache	Englisch
Seiten (von - bis)	30-45
Seitenumfang	16
Fachzeitschrift	Journal of Magnetic Resonance
Jahrgang	280
DOIs	https://doi.org/10.1016/j.jmr.2017.02.023
Publikationsstatus	Veröffentlicht - Juli 2017

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10.1016/j.jmr.2017.02.023

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title = "Perspectives of shaped pulses for EPR spectroscopy",

abstract = "This article describes current uses of shaped pulses, generated by an arbitrary waveform generator, in the field of EPR spectroscopy. We show applications of sech/tanh and WURST pulses to dipolar spectroscopy, including new pulse schemes and procedures, and discuss the more general concept of optimum-control-based pulses for applications in EPR spectroscopy. The article also describes a procedure to correct for experimental imperfections, mostly introduced by the microwave resonator, and discusses further potential applications and limitations of such pulses.",

keywords = "Adiabatic pulses, Dipolar EPR spectroscopy, OCT pulses, Optimum control pulses, Shaped pulses",

author = "Spindler, {Philipp E.} and Philipp Sch{\"o}ps and Wolfgang Kallies and Glaser, {Steffen J.} and Prisner, {Thomas F.}",

note = "Publisher Copyright: {\textcopyright} 2017 Elsevier Inc.",

year = "2017",

month = jul,

doi = "10.1016/j.jmr.2017.02.023",

language = "English",

volume = "280",

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AU - Spindler, Philipp E.

AU - Schöps, Philipp

AU - Kallies, Wolfgang

AU - Glaser, Steffen J.

AU - Prisner, Thomas F.

PY - 2017/7

Y1 - 2017/7

N2 - This article describes current uses of shaped pulses, generated by an arbitrary waveform generator, in the field of EPR spectroscopy. We show applications of sech/tanh and WURST pulses to dipolar spectroscopy, including new pulse schemes and procedures, and discuss the more general concept of optimum-control-based pulses for applications in EPR spectroscopy. The article also describes a procedure to correct for experimental imperfections, mostly introduced by the microwave resonator, and discusses further potential applications and limitations of such pulses.

AB - This article describes current uses of shaped pulses, generated by an arbitrary waveform generator, in the field of EPR spectroscopy. We show applications of sech/tanh and WURST pulses to dipolar spectroscopy, including new pulse schemes and procedures, and discuss the more general concept of optimum-control-based pulses for applications in EPR spectroscopy. The article also describes a procedure to correct for experimental imperfections, mostly introduced by the microwave resonator, and discusses further potential applications and limitations of such pulses.

KW - Adiabatic pulses

KW - Dipolar EPR spectroscopy

KW - OCT pulses

KW - Optimum control pulses

KW - Shaped pulses

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AN - SCOPUS:85020009873

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VL - 280

SP - 30

EP - 45

JO - Journal of Magnetic Resonance

JF - Journal of Magnetic Resonance

ER -

Perspectives of shaped pulses for EPR spectroscopy

Abstract

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