Broadband inversion PELDOR spectroscopy with partially adiabatic shaped pulses

Philipp E. Spindler; Steffen J. Glaser; Thomas E. Skinner; Thomas F. Prisner

doi:10.1002/anie.201207777

Broadband inversion PELDOR spectroscopy with partially adiabatic shaped pulses

Philipp E. Spindler
, Steffen J. Glaser
, Thomas E. Skinner
, Thomas F. Prisner

Professur für Organische Chemie

Johann Wolfgang Goethe University
Wright State University

Publikation: Beitrag in Fachzeitschrift › Artikel › Begutachtung

119 Zitate (Scopus)

Abstract

Distance and spins: A new broadband, frequency-selective inversion pulse has been devised for pulsed electron-electron double resonance (PELDOR) spectroscopy, a unique method used to determine distance distributions between two or more paramagnetic centers 2-10 nm apart. The PELDOR modulation depth can be increased by substituting the rectangular pump pulse by a shaped pulse.

Originalsprache	Englisch
Seiten (von - bis)	3425-3429
Seitenumfang	5
Fachzeitschrift	Angewandte Chemie International Edition in English
Jahrgang	52
Ausgabenummer	12
DOIs	https://doi.org/10.1002/anie.201207777
Publikationsstatus	Veröffentlicht - 18 März 2013

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10.1002/anie.201207777

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abstract = "Distance and spins: A new broadband, frequency-selective inversion pulse has been devised for pulsed electron-electron double resonance (PELDOR) spectroscopy, a unique method used to determine distance distributions between two or more paramagnetic centers 2-10 nm apart. The PELDOR modulation depth can be increased by substituting the rectangular pump pulse by a shaped pulse.",

keywords = "EPR spectroscopy, PELDOR, adiabatic pulses, broadband inversion pulses, transition-metal ions",

author = "Spindler, \{Philipp E.\} and Glaser, \{Steffen J.\} and Skinner, \{Thomas E.\} and Prisner, \{Thomas F.\}",

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AU - Skinner, Thomas E.

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AB - Distance and spins: A new broadband, frequency-selective inversion pulse has been devised for pulsed electron-electron double resonance (PELDOR) spectroscopy, a unique method used to determine distance distributions between two or more paramagnetic centers 2-10 nm apart. The PELDOR modulation depth can be increased by substituting the rectangular pump pulse by a shaped pulse.

KW - EPR spectroscopy

KW - PELDOR

KW - adiabatic pulses

KW - broadband inversion pulses

KW - transition-metal ions

UR - https://www.scopus.com/pages/publications/84875193617

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Broadband inversion PELDOR spectroscopy with partially adiabatic shaped pulses

Abstract

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